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Pulsed laser deposition and magnetron sputtering methods [9, 10]. Therefore, it is feasible to experimentally elucidate various intrinsic optical and thermal properties of these films, including the complex dielectric functions, the tetragonal-to-cubic structural phase transition, and the thermal conductivity [10,11,12]. However, the electric transport measurements of previous (111)-oriented VN thin films on \(\alpha\)-Al\(_2\)O\(_3\)(0001) substrates were only conducted down to a temperature of 10 K [9]. As a result, it remains uncertain whether superconductivity is present in these films or not. Additionally, there are currently no reports on the temperature-dependent electronic structure of VN.To tackle the aforementioned issue, high-quality VN(111) epitaxial films were synthesized on (0001)-Al\(_2\)O\(_3\) single crystal substrates (\(5\times 5 \times 0.5\) mm\(^3\)) by high-pressure magnetron sputtering. The crystal and electronic structures of VN films were characterized by employing a combination of high-resolution X-ray diffraction (XRD), low-energy electron diffraction (LEED), resonant soft X-ray absorption spectroscopy (XAS), and ultraviolet photoelectron spectroscopy (UPS). The electrical transport measurements reveal that the superconducting critical temperature of the VN films is near 8.1 K.Fig. 1Crystal structure of VN films. a Wide-range 2\(\theta\)-\(\omega\) scan of VN/Al\(_2\)O\(_3\)(0001). The black triangles indicate the (111) and (222) peaks of VN films. The inset is the schematic of the VN crystal structure. b XRR (dots) and the fitted curves (solid line) of VN films. c Rocking curve recorded around VN(111) diffractions. d Phi scans of VN/Al\(_2\)O\(_3\)(0001) around VN (200) diffraction and Al\(_2\)O\(_3\) (024) diffraction. e RSM patterns of VN/Al\(_2\)O\(_3\)(0001) around Al\(_2\)O\(_3\) (119) diffraction and VN (113) diffractionFull size image2 Results

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AbstractVanadium nitride (VN) is a transition-metal nitride with remarkable properties that have prompted extensive experimental and theoretical investigations in recent years. However, there is a current paucity of experimental research investigating the temperature-dependent electronic structure of single-crystalline VN. In this study, high-quality VN(111) films were successfully synthesized on \(\alpha\)-Al\(_2\)O\(_3\)(0001) substrates using magnetron sputtering. The crystal and electronic structures of the VN films were characterized by a combination of high-resolution X-ray diffraction, low-energy electron diffraction, resonant soft X-ray absorption spectroscopy, and ultraviolet photoelectron spectroscopy. The electrical transport measurements indicate that the superconducting critical temperature of the VN films is around 8.1 K. Intriguingly, the temperature-dependent photoelectron spectroscopy measurements demonstrate a weak temperature dependence in the electronic structure of the VN films, which is significant for understanding the ground state of VN compounds. Similar content being viewed by others 1 IntroductionDue to the emergence of various extraordinary properties, the study of vanadium-based compounds, such as VO\(_2\), VSe\(_2\), SrVO\(_3\), CsV\(_3\)Sb\(_5\), have recently garnered significant attention [1,2,3,4]. Among these compounds, vanadium nitride (VN) exhibits an excellent combination of high thermal and chemical stability, superconductivity, and high hardness, making it widely applicable in multifunctional coatings, catalysis, and supercapacitors [5,6,7]. More interestingly, VN films can be ideal parent compounds to prepare high-quality and superior-performing VO\(_2\) films [8]. To comprehensively understand the intrinsic properties of VN compounds, it is necessary to synthesize single-crystalline VN films and conduct high-resolution measurements of their electronic structure.With the advancements in film deposition techniques, single-crystalline VN films have been successfully synthesized using